Catalytic oxidative coupling of methane with a dark current in an electric field at low external temperature

K. Oshima, K. Tanaka, T. Yabe, Y. Tanaka, Y. Sekine*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

17 Citations (Scopus)

Abstract

Oxidative coupling of methane (OCM) assisted by a dark current in an electric field was investigated at low external temperature (423 K). The Sr-La2O3 catalyst showed higher yield of C2 (C2H4, C2H6) in the electric field than in the conventional catalytic reaction. Catalytic properties in the electric field and electrical properties of the catalyst were investigated. Results show that the electrical conductivity of dark current of the catalyst is an important factor for applying the electric field. A higher CH4/O2 ratio enabled high selectivity to C2 hydrocarbons. The maximum selectivity to C2 hydrocarbons was 59%.

Original languageEnglish
Pages (from-to)266-271
Number of pages6
JournalInternational Journal of Plasma Environmental Science and Technology
Volume6
Issue number3
Publication statusPublished - 2012 Dec 1

Keywords

  • Catalytic reaction
  • Dark current
  • Electric field
  • Natural gas conversion

ASJC Scopus subject areas

  • Environmental Science(all)

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