TY - JOUR
T1 - Direct detection and stochastic analysis on thermally activated domain-wall depinning events in micropatterned Nd-Fe-B hot-deformed magnets
AU - Yomogita, Takahiro
AU - Okamoto, Satoshi
AU - Kikuchi, Nobuaki
AU - Kitakami, Osamu
AU - Sepehri-Amin, Hossein
AU - Takahashi, Yukiko K.
AU - Ohkubo, Tadakatsu
AU - Hono, Kazuhiro
AU - Hioki, Keiko
AU - Hattori, Atsushi
N1 - Funding Information:
We gratefully thank S. Hirosawa, A. Sakuma, Y. Toga, S. Miyashita for fruitful discussions. The FIB patterning was performed at Material Solution Center (MaSC), Tohoku Univ. with great supports by K. Sato. This work was partially supported by Dynamic Alliance for Open Innovation Bridging Human, Environment and Materials, MEXT, the Management Expenses Grants for National Universities Corporations , MEXT , JSPS KAKENHI grant no. 17H03376 , and ESICMM grant no. JPMXP0112101004 , MEXT.
Publisher Copyright:
© 2020
PY - 2020/12
Y1 - 2020/12
N2 - Although the magnetization reversal process in the permanent magnets has long been studied, it has not been fully revealed. The recent progress of the computational science realizes the atomistic calculations for the thermally activated magnetization reversal process in permanent magnets. In contrast, the experimental study on the magnetization reversal has remain to be the macroscopic evaluation. In this study, Nd-Fe-B hot-deformed magnets are micropatterned, and a staircase-like magnetization curve corresponding to the elemental domain-wall depinning event at each grain boundary is successfully observed. Each elemental domain-wall depinning event fluctuates with respect to thermal activation, and the stochastic analysis based on the Néel-Arrhenius model gives the energy barrier parameters H0 and E0 of each depinning event, which are the intrinsic domain-wall depinning field and energy barrier height, respectively. Three types of Nd-Fe-B hot-deformed magnets with different coercivities are adopted for this stochastic analysis. As a result, E0 exhibits very little dependence on H0, and its slope becomes steeper for the lower-coercivity magnet. The stochastic micromagnetics simulation based on the Landau-Lifshitz-Gilbert equation for the two-grain model with various inter-grain exchange coupling reproduces the experimentally observed relationship between E0 and H0. Moreover, the behavior for the lower-coercivity magnet can be explained by assuming the presence of a low magnetic anisotropy layer on the grain surface.
AB - Although the magnetization reversal process in the permanent magnets has long been studied, it has not been fully revealed. The recent progress of the computational science realizes the atomistic calculations for the thermally activated magnetization reversal process in permanent magnets. In contrast, the experimental study on the magnetization reversal has remain to be the macroscopic evaluation. In this study, Nd-Fe-B hot-deformed magnets are micropatterned, and a staircase-like magnetization curve corresponding to the elemental domain-wall depinning event at each grain boundary is successfully observed. Each elemental domain-wall depinning event fluctuates with respect to thermal activation, and the stochastic analysis based on the Néel-Arrhenius model gives the energy barrier parameters H0 and E0 of each depinning event, which are the intrinsic domain-wall depinning field and energy barrier height, respectively. Three types of Nd-Fe-B hot-deformed magnets with different coercivities are adopted for this stochastic analysis. As a result, E0 exhibits very little dependence on H0, and its slope becomes steeper for the lower-coercivity magnet. The stochastic micromagnetics simulation based on the Landau-Lifshitz-Gilbert equation for the two-grain model with various inter-grain exchange coupling reproduces the experimentally observed relationship between E0 and H0. Moreover, the behavior for the lower-coercivity magnet can be explained by assuming the presence of a low magnetic anisotropy layer on the grain surface.
KW - Domain-wall depinning
KW - Magnetization reversal
KW - Nd-Fe-B magnet
KW - Thermal activation
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U2 - 10.1016/j.actamat.2020.09.074
DO - 10.1016/j.actamat.2020.09.074
M3 - Article
AN - SCOPUS:85092049832
SN - 1359-6454
VL - 201
SP - 7
EP - 13
JO - Acta Materialia
JF - Acta Materialia
ER -