TY - JOUR
T1 - Nd isotopic composition in the central North Pacific
AU - Amakawa, Hiroshi
AU - Sasaki, Kazunori
AU - Ebihara, Mitsuru
N1 - Funding Information:
We are grateful to the captain, officers, and crew of the R.V. Hakuho-Maru, and to the scientific parties of the “Bootes” Expeditions for their collaboration in sampling. We thank Dr. H. Tazoe for collecting the KH-08-2 sample. We also thank Associate Editor Mark Rehkämper for handling the manuscript and A. Piotrowski and two anonymous reviewers for their useful and constructive comments. This work was supported in part by Ministry of Education, Culture, Sports, Science and Technology (MEXT) Grants-in-Aid No. 15540466 (P.I. Hiroshi Amakawa) to the Ocean Research Institute, University of Tokyo and No. 15340193 (P.I. Mitsuru Ebihara) to Tokyo Metropolitan University.
PY - 2009/8/15
Y1 - 2009/8/15
N2 - Three vertical profiles of seawater concentration and isotopic composition of Nd were determined for the western to central North Pacific Ocean. In the subarctic oceanic region, at depths greater than 500 m, one vertical profile of Nd isotopic composition was indistinguishable from most previously reported profiles from here. The data indicate a rather homogeneous Nd isotopic composition in the subarctic oceanic region at middle to deep depths (>500 m). Two stations in the subtropical oceanic region exhibited similar Nd isotopic composition profiles to those previously reported. The maxima εNd values at depths of 800-1000 m (εNd = -3.4 to -2.7), which correspond to the North Pacific Intermediate Water (NPIW), are found at both subtropical stations. This implies a ubiquitous distribution of NPIW showing a radiogenic εNd value in the North Pacific. The subsurface minimum at a depth of ∼200 m, which indicates the penetration of the North Pacific Tropical Water (NPTW) with an unradiogenic Nd isotopic signal, was observed at one station in the western Pacific. This station had much lower εNd than the central station at depths around 5000 m, suggesting the greater prominence of Antarctic Bottom Water (AABW) in the western subtropical Pacific than in the central to eastern subtropical Pacific. Results of a model calculation assuming boundary exchange indicate that the Hawaiian Islands play an important role in supplying radiogenic Nd to the central Pacific, similar to some continental margins. We show that Nd isotopic composition is a versatile tracer for ocean circulation and the geochemical cycle of Nd in the North Pacific. Further studies on the distribution of Nd isotopic composition in the Pacific Ocean, including the Southern Pacific, will better elucidate the circulation and geochemical cycle of Nd in the Pacific.
AB - Three vertical profiles of seawater concentration and isotopic composition of Nd were determined for the western to central North Pacific Ocean. In the subarctic oceanic region, at depths greater than 500 m, one vertical profile of Nd isotopic composition was indistinguishable from most previously reported profiles from here. The data indicate a rather homogeneous Nd isotopic composition in the subarctic oceanic region at middle to deep depths (>500 m). Two stations in the subtropical oceanic region exhibited similar Nd isotopic composition profiles to those previously reported. The maxima εNd values at depths of 800-1000 m (εNd = -3.4 to -2.7), which correspond to the North Pacific Intermediate Water (NPIW), are found at both subtropical stations. This implies a ubiquitous distribution of NPIW showing a radiogenic εNd value in the North Pacific. The subsurface minimum at a depth of ∼200 m, which indicates the penetration of the North Pacific Tropical Water (NPTW) with an unradiogenic Nd isotopic signal, was observed at one station in the western Pacific. This station had much lower εNd than the central station at depths around 5000 m, suggesting the greater prominence of Antarctic Bottom Water (AABW) in the western subtropical Pacific than in the central to eastern subtropical Pacific. Results of a model calculation assuming boundary exchange indicate that the Hawaiian Islands play an important role in supplying radiogenic Nd to the central Pacific, similar to some continental margins. We show that Nd isotopic composition is a versatile tracer for ocean circulation and the geochemical cycle of Nd in the North Pacific. Further studies on the distribution of Nd isotopic composition in the Pacific Ocean, including the Southern Pacific, will better elucidate the circulation and geochemical cycle of Nd in the Pacific.
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U2 - 10.1016/j.gca.2009.05.058
DO - 10.1016/j.gca.2009.05.058
M3 - Article
AN - SCOPUS:67650083178
SN - 0016-7037
VL - 73
SP - 4705
EP - 4719
JO - Geochmica et Cosmochimica Acta
JF - Geochmica et Cosmochimica Acta
IS - 16
ER -