Chemical species of localized fe atoms in solid hydrogen using in-beam mössbauer spectroscopy

Yoshio Kobayashi*, Masami Sato, Yasuhiro Yamada, Michael K. Kubo, Mototsugu Mihara, Wataru Sato, Takashi Nagatomo, Jun Miyazaki, Atsushi Okazawa, Shinji Sato, Atsushi Kitagawa

*この研究の対応する著者

研究成果: Article査読

抄録

The 57Fe Mössbauer spectrum obtained after 57Mn (T1/2 = 1.45 min) implantation of solid hydrogen was measured at 7 K. The spectrum was analyzed as three components, and the chemical species of each component was assigned from the obtained Mössbauer parameters and the results of density functional theory (DFT) calculations. The formation process of chemical species and the oxidation states of Fe atoms produced by β decay of 57Mn are discussed considering the charge transfer process, in relation to previous emission Mössbauer spectroscopy experiments with 57Co implantation of solid hydrogen at low temperature.

本文言語English
論文番号13
ジャーナルHyperfine Interactions
243
1
DOI
出版ステータスPublished - 2022 12月
外部発表はい

ASJC Scopus subject areas

  • 原子分子物理学および光学
  • 核物理学および高エネルギー物理学
  • 凝縮系物理学
  • 物理化学および理論化学

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