Key factor for the anti-Arrhenius low-temperature heterogeneous catalysis induced by H+ migration: H+ coverage over support

Kota Murakami; Yuta Tanaka; Ryuya Sakai; Yudai Hisai; Sasuga Hayashi; Yuta Mizutani; Takuma Higo; Shuhei Ogo; Jeong Gil Seo; Hideaki Tsuneki; Yasushi Sekine

doi:10.1039/d0cc00482k

Key factor for the anti-Arrhenius low-temperature heterogeneous catalysis induced by H⁺ migration: H⁺ coverage over support

Kota Murakami, Yuta Tanaka, Ryuya Sakai, Yudai Hisai, Sasuga Hayashi, Yuta Mizutani, Takuma Higo, Shuhei Ogo, Jeong Gil Seo, Hideaki Tsuneki, Yasushi Sekine^*

^*この研究の対応する著者

研究成果: Article › 査読

28 被引用数 (Scopus)

抄録

Low-temperature heterogeneous catalytic reaction in an electric field is anticipated as a novel approach for on-demand and small-scale catalytic processes. This report quantitatively reveals the important role of proton coverage on the catalyst support for catalytic ammonia synthesis in an electric field, which shows an anti-Arrhenius behaviour.

本文言語	English
ページ（範囲）	3365-3368
ページ数	4
ジャーナル	Chemical Communications
巻	56
号	23
DOI	https://doi.org/10.1039/d0cc00482k
出版ステータス	Published - 2020 3月 21

ASJC Scopus subject areas

触媒
電子材料、光学材料、および磁性材料
セラミックおよび複合材料
化学一般
表面、皮膜および薄膜
金属および合金
材料化学

文献へのアクセス

10.1039/d0cc00482k

他のファイルとリンク

引用スタイル

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author = "Kota Murakami and Yuta Tanaka and Ryuya Sakai and Yudai Hisai and Sasuga Hayashi and Yuta Mizutani and Takuma Higo and Shuhei Ogo and Seo, {Jeong Gil} and Hideaki Tsuneki and Yasushi Sekine",

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AU - Murakami, Kota

AU - Tanaka, Yuta

AU - Sakai, Ryuya

AU - Hisai, Yudai

AU - Hayashi, Sasuga

AU - Mizutani, Yuta

AU - Higo, Takuma

AU - Ogo, Shuhei

AU - Seo, Jeong Gil

AU - Tsuneki, Hideaki

AU - Sekine, Yasushi

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AB - Low-temperature heterogeneous catalytic reaction in an electric field is anticipated as a novel approach for on-demand and small-scale catalytic processes. This report quantitatively reveals the important role of proton coverage on the catalyst support for catalytic ammonia synthesis in an electric field, which shows an anti-Arrhenius behaviour.

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