Pd-Catalyzed Alkenyl Thioether Synthesis from Thioesters and N-Tosylhydrazones

Kota Ishitobi, Kei Muto, Junichiro Yamaguchi*

*この研究の対応する著者

研究成果: Article査読

28 被引用数 (Scopus)

抄録

A Pd-catalyzed alkenyl thioether synthesis was achieved using thioesters and N-tosylhydrazones as starting materials. The thioester acted as an efficient "sulfur source" for catalytic C-S bond formation using N-tosylhydrazone. This method gave Z-alkenyl thioethers with high diastereoselectivity (up to 99:1 diastereomeric ratio). This transformation displayed a wide functional group tolerance and was successfully applied to the late-stage derivatization of a pharmaceutical molecule to the corresponding alkenyl thioether.

本文言語English
ページ(範囲)11685-11690
ページ数6
ジャーナルACS Catalysis
9
12
DOI
出版ステータスPublished - 2019 12月 6

ASJC Scopus subject areas

  • 触媒
  • 化学 (全般)

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