Relativistic local hybrid functionals and their impact on 1s core orbital energies

Toni M. Maier, Yasuhiro Ikabata, Hiromi Nakai, Hiromi Nakai

研究成果: Article査読

7 被引用数 (Scopus)

抄録

In this work, we report the first relativistic density functional theory calculations using relativistic local hybrid functionals. Besides outlining the construction of relativistic local hybrid exchange within a two-component-relativistic framework based on the picture-change transformation of the density matrix and a recently developed relativistic iso-orbital indicator, we investigate the influence of two-electron-relativistic effects, using relativistic functional ingredients in local hybrid functionals, and the choice of the exchange-correlation functional on atomic 1s core orbital energies of light and heavier elements. Finally, we discuss the applicability of relativistic 1s core orbital shifts for the relativistic correction of non-relativistic 1s core excitation energies.

本文言語English
論文番号0010400
ジャーナルJournal of Chemical Physics
152
21
DOI
出版ステータスPublished - 2020 6月 7

ASJC Scopus subject areas

  • 物理学および天文学(全般)
  • 物理化学および理論化学

フィンガープリント

「Relativistic local hybrid functionals and their impact on 1s core orbital energies」の研究トピックを掘り下げます。これらがまとまってユニークなフィンガープリントを構成します。

引用スタイル